Frontiers in operando and in situ soft X-ray spectroscopy

- A workshop of 2017 Advanced Light Source Users Meeting

Organizers: Hendrik Bluhm, Ethan Crumlin, Jinghua Guo, Wanli Yang

Time: October 3, 1:30PM - October 4, 18:00PM 2017 (PCT)
Location: Lawrence Berkeley National Laborotary (Travel and Site Access)
Lodging: Berkeley Lab Guest House
Conference Room: Building 50 Auditorium

Heterogeneous interfaces govern some of the most important processes in such diverse areas as catalysis, electrochemistry, and environmental science.  Soft X-ray spectroscopies, including XPS, NEXAFS, and RIXS, are excellent tools to investigate these interfaces with high elemental and chemical sensitivity. This workshop will highlight recent developments in the application of soft X-ray spectroscopies under reaction conditions, including the design of new experimental strategies for the preparation and control of liquid/solid, gas/solid and liquid/vapor interfaces.

 

Agenda

Tuesday, Oct 3, 2017

08:00 – 11:50               ALS User Meeting – General Program

11:50 – 13:20               Lunch

 

Session I

13:20                            Opening remarks

13:30                            Miquel Salmeron

                                    The electrical double layer as seen from the electrode side by XAS

14:00                            David Prendergast

                                    Understanding what X-ray spectroscopy can tell us about buried interfaces

14:30                            Lothar Weinhardt

In situ soft x-ray spectroscopy of biologically relevant systems in solution

                       

15:00 – 15:30               Coffee Break

 

Session II

15:20                            Shawn Sallis

                                    Analysis of Operando and In-Situ Spectroscopy Data Using Blind Source Separation and Bayesian Inference

15:40                            Lena Trotochaud

Quick-and-Dirty No More: Quantification of Surface Carbon in APXPS Experiments

16:00                            Ruimin Qiao

                                    Soft x-ray spectroscopy of high pressure liquid

16:20                            Carlos Valero

                                    Corrosion mechanism of titanium in presence of fluorides determined in operando by ambient pressure XPS

16:40                            Timm Gerber

A Setup for core level spectroscopy of Langmuir films at the liquid-vapor interface

 

17:00 – 19:00               Awards Dinner, ALS Patio

 

 

Wednesday, Oct 4, 2017

08:00 – 08:30               Breakfast, ALS Patio

 

Session III

08:30                            Michael Toney

Soft X-ray spectroscopy and spectro-microscopy in Li-ion energy storage electrodes

09:00                            Anibal Boscoboinik

Exploring 2D-Nanoporous Materials with APXPS

09:30                            Ashley Head

                                    Multimodal IR and APXPS: First Results and Potential for the Future

 

10:00 – 10:30               Coffee Break

 

Session IV

10:30                            Kelsey Stoerzinger
Understanding the surface of perovskite oxides during oxygen electrocatalysis

11:00                            Oleg Kostko

                                    Spectroscopy and dynamics in nanoparticles

11:30                            Dunwei Wang
Understanding what limits the performance of hematite-based water splitting using soft X-ray absorption spectroscopy

 

12:00 – 13:30               Lunch Break

 

Session V

13:30                            Liang Zhang   

                                    Application of operando X-ray spectroscopy in lithium-sulfur batteries

14:00                            Monika Blum

                                    In situ/Operando Measurements of Energy Materials Studied by Soft and Tender X-ray Spectroscopies

14:30                            Matthew Roberts

                                    Studying Oxygen Redox in Li-Ion Battery Chemistries

 

15:00 – 15:30               Coffee Break

 

Session VI

15:30                            Francesca Toma

Towards in situ and operando characterization of photoelectrochemical assemblies

16:00                            Christian Kisielowski

Modulating electron beams in space and time to probe for genuine structures and function at the atomic scale

16:30                            Junko Yano

Capturing Reaction Intermediates in Metalloenzymes and Catalysts with Soft X-ray Spectroscopy

                                   

17:00-18:00 ---------------------------------------------------------------------- Adjourn